Optimal Magneto‐Optical Angle in Single‐Beam Optically Pumped Atomic Magnetometers Considering the Spatial Distribution of Spin Polarization

ABSTRACT Single‐beam optically pumped atomic magnetometers (OPAMs) are promising tools for biomagnetic measurements in nonzero‐field environments owing to their high sensitivity and compactness. However, the angle between the external bias magnetic field and the pump light affects the spin polarization of the atomic ensemble, thereby influencing the magnetometer performance and making the optimization of the magneto‐optical angle essential. In this study, a spatially resolved steady‐state spin polarization model incorporating the magneto‐optical angle is established for the first time, and an analytical expression of the spin precession signal under RF magnetic field excitation is derived. It is demonstrated that an optimal angle exists at which the magnetometer exhibits the maximum response and the highest sensitivity, which is experimentally determined to be 26° in our single‐beam OPAM. At this angle, the combined influence of the steady‐state spin polarization, spin precession projection, transmitted light intensity, and transverse spin relaxation reaches an optimal overall state, leading to a 14% enhancement in sensitivity and a 32% reduction in detection noise compared with the conventional 45° configuration. These findings provide guidance for optimizing the experimental parameters of single‐beam OPAMs for weak magnetic signal detection in nonzero‐field environments.