Zero-phonon line emission of single photon emitters in helium-ion treated MoS$_2$

Read full text
Authors: Katja Barthelmi, Tomer Amit, Mirco Troue, Lukas Sigl, Alexander Musta, Tim Duka, Samuel Gyger, Val Zwiller, Matthias Florian, Michael Lorke, Takashi Taniguchi, Kenji Watanabe
+4 more Christoph Kastl, Jonathan Finley, Sivan Refaely‐Abramson, Alexander W. Holleitner
Cited by: 0

Abstract

We explore the zero-phonon line of single photon emitters in helium-ion treated monolayer MoS$_2$, which are currently understood in terms of single sulfur-site vacancies. By comparing the linewidths of the zero-phonon line as extracted directly from optical spectra with values inferred from the first-order autocorrelation function of the photoluminescence, we quantify bounds of the homogeneous broadening and of phonon-assisted contributions. The results are discussed in terms of both the independent boson model and ab-initio results as computed from GW and Bethe-Salpeter equation approximations.

Fields of Study & Subjects

2D Materials and Applications Semiconductor Quantum Structures and Devices Graphene research and applications

Publication details

Journal / source
arXiv (Cornell University)
Publication date
18 January 2026
Document type
Preprint