SUBFEMTOSECOND DELAY OF THE CUBIC NONLINEARITY OF GASEOUS MEDIA
Abstract
We establish the physical mechanism of the long-wavelength spectral shift during the propagation of an ultraviolet femtosecond pulse in gases using a numerical solution of the non-stationary Schrödinger equation. It is shown that the source of long-wavelength radiation is the leading edge of the pulse, where a cubic response delayed by approximately 100 as develops with a nearly zero phase shift between the polarization and the pump field. It was established that the long-wavelength shift of the spectrum arises due to the superposition of contributions from bound-bound and bound-free transitions.
Fields of Study & Subjects
Laser-Matter Interactions and Applications
Photorefractive and Nonlinear Optics
Photonic Crystal and Fiber Optics
Publication details
- Journal / source
- Radiophysics and Quantum Electronics
- Volume
- 69
- Issue
- 1
- Pages
- 82–82
- Publication date
- 1 January 2026
- Language
- EN