Low-Dimensionality-Induced Tunable Ferromagnetism in SrRuO 3 Ultrathin Films

Quantum materials near electronic or magnetic phase boundaries exhibit enhanced tunability as their emergent properties become highly sensitive to external perturbations. Here, we demonstrate precise control of ferromagnetism in a SrRuO 3 ultrathin film, where a high density of states (DOS), arising from low-dimensional quantum states, places the system at the crossover between a nonmagnetic and bulk ferromagnetic state. Using spin- and angle-resolved photoemission spectroscopy (SRPES/ARPES), transport measurements, and theoretical calculations, we systematically tune the Fermi level via electron doping across the high-DOS point. We directly visualize the spin-split band structure and reveal its influence on both the magnetic and transport properties. Our findings provide compelling evidence that magnetism can be engineered through DOS control at a phase crossover, establishing a pathway for the rational design of tunable quantum materials.