In-Silicon Mietronics for Flatband-Enhanced Upconversion and Interfacial Loss Recovery
Abstract
Silicon (Si) photodetectors exhibit limited infrared responsivity, restricting applications in communication, chemical sensing, and biomedical imaging. Although lanthanide-doped upconversion nanoparticles (UCNPs) can extend the spectral response of silicon, weak IR absorption and interfacial nonradiative losses have hindered etch-free monolithic integration. Here, we report an inverted-index UCNP-Si metasurface in which low-index NaYF 4:Yb/Er nanocylinders are conformally coated with a high-index amorphous silicon layer. A collective-Mie flatband resonance at 976 nm enables near-unity absorption, simultaneously concentrating pump photons within the UCNP domains over a wide numerical aperture (NA ≈ 0.5) and activating near-field-mediated passivation of interfacial loss channels. The combined effects of resonant field enhancement and light-activated loss recovery yield a record 6800-fold increase in long-lived steady-state upconversion. This fully etch-free platform is compatible with complementary metal oxide semiconductor processing and provides a scalable route toward upconversion-enabled silicon photodetectors and compact light sources.
Fields of Study & Subjects
Luminescence Properties of Advanced Materials
Silicon Nanostructures and Photoluminescence
Thermal Radiation and Cooling Technologies
Publication details
- Journal / source
- Nano Letters
- Publisher
- American Chemical Society (ACS)
- Volume
- 26
- Issue
- 9
- Pages
- 3291–3297
- Publication date
- 2 March 2026
- Language
- EN