Many-Body Exciton Interactions, Coherence, and Transport in Perovskite Quantum Dots

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Authors: Kinjol Barua, Sonja G. Nusser, Shriya Gumber, Nicholas Favate, Emma Daggett, Meng‐Jia Sun, Jonathan D. Hood, Jianshu Cao, Christina W. Li, Oleg V. Prezhdo, Libai Huang
Cited by: 1
References: 98

Abstract

Realizing robust many-body exciton interactions, coherence, and long-range exciton transport is central to technologies ranging from quantum information science (QIS) to light-emitting devices and solar cells. Colloidal quantum dots (QDs) offer scalable fabrication and spectral tunability, yet performance is suppressed by inhomogeneous broadening, defects, and fast dephasing. Lead-halide perovskite QDs, exhibiting large transition dipole moments, high radiative efficiencies, and slow low-temperature dephasing, enable strong light-matter coupling and long-range dipolar exciton-exciton interactions. This review focuses on the origins and consequences of many-body exciton physics in perovskite QDs, including dipole-mediated interactions and cooperative radiative phenomena. We discuss how exciton fine structure, inter-QD electronic coupling, and exciton-phonon interactions govern coherence and the role of disorder. We then examine exciton transport in QD solids, emphasizing the crossover from coherent motion enabled by delocalized excitonic wave functions to dephasing-driven incoherent hopping. Finally, we survey routes toward scalable many-body states through nanophotonic integration.

Fields of Study & Subjects

Perovskite Materials and Applications Strong Light-Matter Interactions Quantum Dots Synthesis And Properties

Publication details

Journal / source
Nano Letters
Publisher
American Chemical Society (ACS)
Volume
26
Issue
21
Pages
6766–6779
Publication date
22 May 2026
Language
EN