Regulation of Energy and Mass Transport in a Hydrogen-Bonded Framework for Visible-Light-Driven CO 2 Reduction in Water

Journal of the American Chemical Society 2026 Open access

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Authors: Jiaxing Xu, Xi Zhang, Lijuan Ma, Tao Wu, Hao Wang, Yuanfang Deng, Jun Xia, Zhongyang Qiu, Kai Sun, Aiyong He, J. Zhang, Xu Zhang
+1 more Banglin Chen
DOI: 10.1021/jacs.6c00570
Cited by: 1
References: 49

Abstract

with 100% selectivity─the highest rate reported to date for all light-driven systems in water. The HOF-based catalyst retains 86.3% of its initial activity over five cycles, highlighting its robustness. This work offers mechanistic insight into how microenvironment engineering within HOF architectures regulates energy and mass transport in photoenzymatic catalysis, paving the way for the rational design of advanced hybrid catalytic systems.

Fields of Study & Subjects

CO2 Reduction Techniques and Catalysts Advanced Photocatalysis Techniques Covalent Organic Framework Applications

Publication details

Journal / source
Journal of the American Chemical Society
Publisher
American Chemical Society (ACS)
Volume
148
Issue
15
Pages
16079–16089
Publication date
8 April 2026
Language
EN