Role of Future Climate Change, Air Pollution Control and Methane Mitigation in Driving Hydroxyl Radical (OH) and Methane Lifetime

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Authors: Glen Chua, Vaishali Naïk, Larry W. Horowitz
Cited by: 0
References: 30

Abstract

Abstract The hydroxyl radical (OH) determines the atmospheric lifetime of many pollutants like methane (). This study isolates climate change, air pollution control and mitigation effects on OH concentrations ([OH]) and lifetime, by analyzing Coupled Model Intercomparison Project Phase 6 (CMIP6) Aerosol Chemistry Model Intercomparison Project (AerChemMIP) multi‐model outputs for variants of the high‐emission SSP3‐7.0 scenario. Models agree that warming increases [OH] and decreases lifetime, leading to a multi‐model mean radiative forcing reduction of −0.038 . However, the overall trend in SSP3‐7.0 is decreasing [OH] and increasing lifetime, confirming that changes in and other short‐lived climate forcers (SLCFs)) dominate over climate‐related drivers. Meanwhile, air pollution controls, if not paired with reduction, can reduce [OH] and lengthen lifetime, potentially undermining climate efforts. In a cleaner‐air future, mitigation will be essential to sustain higher [OH], shorten lifetime, and reduce its radiative forcing.

Fields of Study & Subjects

Atmospheric chemistry and aerosols Atmospheric and Environmental Gas Dynamics Odor and Emission Control Technologies

Publication details

Journal / source
Geophysical Research Letters
Volume
53
Issue
9
Publication date
6 May 2026
Language
EN