Sonochemical synthesis of robust covalent organic frameworks via one-pot Doebner reactions in aqueous media

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Authors: Kun Wu, Ling Huang, Jia-Yu Huang, Wen-Ting Zeng, Weigang Lu, Dan Li
Cited by: 1
References: 32

Abstract

Here, we report a facile and sustainable strategy for converting imine linkages to dihydroquinoline-4-carboxylic acid linkages without compromising the framework integrity. One-pot aqueous-phase three-component Doebner reactions of aromatic dialdehydes, pyrene-based tetraamine, and pyruvic acid under ultrasonic irradiation afford highly crystalline COFs. The resulting functionalized COFs can promote photocatalytic aerobic oxidation.

Fields of Study & Subjects

Covalent Organic Framework Applications Multicomponent Synthesis of Heterocycles Supramolecular Chemistry and Complexes

Publication details

Journal / source
Chemical Communications
Publisher
Royal Society of Chemistry (RSC)
Volume
62
Issue
22
Pages
6200–6204
Publication date
1 January 2026
Language
EN