RKKY-Dipolar Interactions and 3D Spin Supersolid on Stacked Triangular Lattice

Abstract Inspired by the recent discovery of metallic spin supersolidity and its giant magnetocaloric effect in the rare-earth alloy EuCo 2 Al 9 , we perform a combined study through electronic structure analysis, effective spin model construction, and Monte Carlo simulations on a stacked triangular lattice (STL), and reveal a novel mechanism for the emergence of 3D spin supersolid in a metallic antiferromagnet. From first-principles inputs, we derive a minimal spin model on a STL, which arises from the interplay between Ruderman–Kittel–Kasuya–Yosida and dipolar interactions and accurately reproduces the experimental thermodynamics. Based on the STL model, we identify a ground state that simultaneously breaks discrete lattice translational symmetry and continuous spin-rotational symmetry—the hallmark of a spin supersolid. Furthermore, we present the field–temperature phase diagram of the 3D STL model and discuss the various magnetic phases and associated phase transitions. Under zero field, the spin supersolid Y order establishes in two steps: an upper transition at T N1 , where an emergent U (1) symmetry appears and the system enters a fluctuating collinear regime, followed by a lower transition at T N2 into the spin supersolid Y phase. In contrast, the supersolid V phase undergoes a single phase transition at T N V . Our results not only provide a comprehensive theoretical understanding of the metallic spin supersolid reported for EuCo 2 Al 9 but also pave the way for further experimental investigations into its supersolid transitions and universality class.