Exchange and spin–orbit proximity-driven topological and transport phenomena in twisted graphene/CrI 3 heterostructures

Abstract We present results of comprehensive first-principles and kp-method studies of electronic, magnetic, and topological properties of graphene on a monolayer of CrI 3 . First, we identify a twist angle between the graphene and CrI 3 , that positions the graphene Dirac cones within the bandgap of CrI 3 . Then, we derive the low-energy effective Hamiltonian describing electronic properties of graphene Dirac cones. Subsequently, we examine anomalous and valley Hall conductivity and discuss possible topological phase transition from a quantum anomalous Hall insulator to a trivial insulating state, concomitant a change in the magnetic ground state of CrI 3 . These findings highlight the potential of strain engineering in two-dimensional van der Waals heterostructures for controlling topological and magnetic phases.