Spectroscopic Demarcation of Emergent Photons and Spinons in a Dipolar-Octupolar Quantum Spin Liquid

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Authors: Bin Gao, Zhengbang Zhou, Tingjun Zhang, Andrey A. Podlesnyak, Sang-Wook Cheong, Yong Baek Kim, Pengcheng Dai
Cited by: 1
References: 60

Abstract

The identification of fractionalized excitations in quantum spin liquids (QSLs) remains a central challenge in condensed matter physics. In dipolar-octupolar (DO) pyrochlores, such as Ce_{2}Zr_{2}O_{7}, the candidate π-flux quantum spin ice (QSI) state is predicted to host both gapless emergent photons and a continuum of spinons. However, resolving these modes at zero field is complicated by their spectral overlap and the presence of nonmagnetic scattering near zero energy. Here, we report neutron scattering experiments on Ce_{2}Zr_{2}O_{7} under a magnetic field along the [1, 1, 1] direction. In contrast to previous unpolarized studies at zero field that relied on high-temperature subtraction, we use a same-temperature high-field subtraction protocol to isolate the photon and spinon modes. Leveraging the selective coupling of the magnetic field to the dipolar degrees of freedom, we demonstrate the spectroscopic demarcation of these excitations. We observe that weak fields (≈0.15 T) suppress the low-energy photon weight while leaving the high-energy spinon continuum robust, albeit hardened. Our results, supported by gauge mean-field theory and exact diagonalization calculations, provide strong evidence for the π-flux QSI state and introduce a powerful field-tuning protocol for investigating DO-QSLs.

Fields of Study & Subjects

Advanced Condensed Matter Physics Topological Materials and Phenomena Physics of Superconductivity and Magnetism

Publication details

Journal / source
Physical Review Letters
Publisher
American Physical Society (APS)
Volume
136
Issue
25
Pages
256703–256703
Publication date
19 May 2026
Language
EN