Cavity Controls Core-to-Core Resonant Inelastic X-Ray Scattering

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Authors: Shu-Xing Wang, Z-Q Zhao, X.-Y. Wang, T. P. Li, Y. Su, Yohei Uemura, Federico Alves Lima, Azat Khadiev, B.-H. Wang, J. M. Ablett, J.-P Rueff, H.-C. Wang
+4 more O. J. L. Fox, W. B. Li, L-F Zhu, Xin‐Chao Huang
Cited by: 0
References: 60

Abstract

X-ray cavity quantum optics with inner-shell transitions has been limited by the spectral overlap between resonant and continuum states. Here, we report the first experimental demonstration of cavity-controlled core-to-core resonant inelastic x-ray scattering (RIXS). We suppress the absorption-edge effects by monitoring the RIXS profile, thereby resolving the resonant state from the overlapping continuum. We observe distinct cavity-induced energy shifts and cavity-enhanced decay rates in the 2p3d RIXS spectra of WSi_{2}. These effects, manifesting as stretched or shifted profiles in the RIXS planes, enable novel spectroscopic applications via cavity-controlled core-hole states. Our results establish core-to-core RIXS as a powerful tool to manipulate inner-shell dynamics in x-ray cavities, offering new avenues for integrating quantum optical effects with x-ray spectroscopy.

Fields of Study & Subjects

Crystallography and Radiation Phenomena Mechanical and Optical Resonators Cold Atom Physics and Bose-Einstein Condensates

Publication details

Journal / source
Physical Review Letters
Volume
136
Issue
6
Pages
063601–063601
Publication date
9 January 2026
Language
EN