Ultrabroadband transient absorption spectroscopy with sub-25 µOD sensitivity and double differential scatter and noise rejection

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Authors: Cooper Johnston, Nicolette Puskar, Isabel Vargas-Hurlston, Kayla Eichmann, Qirui Wang, Arnav Modak, Jwwad Javed, Ashley Arcidiacono, Sarah King
Cited by: 1
References: 48

Abstract

Transient absorption spectroscopy is a powerful technique for studying charge transfer, energy conversion, and electron-phonon coupling in an array of chemical and material systems on the femtosecond to nanosecond timescales. Here, we describe a state-of-the-art ultrabroadband transient absorption spectrometer for solid samples, which achieves sub-50 fs time resolution and sub-25 µOD sensitivity across a wide spectral range, from 350 to 900 nm. Combined with suppression of pump pulse scatter, the high signal-to-noise ratio of this spectrometer allows investigating previously inaccessible phenomena in well studied samples, such as electron-phonon coupling signatures in transition metal oxides.

Fields of Study & Subjects

Spectroscopy and Laser Applications Spectroscopy and Quantum Chemical Studies Spectroscopy Techniques in Biomedical and Chemical Research

Publication details

Journal / source
Optics Express
Publisher
Optica Publishing Group
Volume
34
Issue
12
Pages
22393–22393
Publication date
19 May 2026
Language
EN