Laser-dressed ionic states in high-harmonic generation in helium

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Authors: Yu He, Eleni Tzima, Gergana Dimitrova Borisova, Lina Hedewig, Noah L. Wach, Harijyoti Mandal, Christian Ott, Thomas Pfeifer
Cited by: 0
References: 51

Abstract

We report the experimental observation of an ionic resonance at 40.8 eV and two adjacent satellite sidebands in high-harmonic generation in neutral helium gas. The amplitude and asymmetry of the central line vary with different driving pulse intensities, which arises from the interference between the laser-dressed resonant emission from the 2 p state of He + ions and the nonresonant harmonic generation. The two satellite sidebands are identified as the virtual Floquet-like light-induced states located at ± ℏ ω d from the 2 s state of He + ions ( ω d denotes the driving laser frequency), whose multipeak profiles are imprinted by the structured spectrum of the driving laser pulse. These results demonstrate the roles of both bright and dark states of ionic species in shaping high-harmonic spectra in the vicinity of resonances.

Fields of Study & Subjects

Laser-Matter Interactions and Applications Atomic and Molecular Physics Spectroscopy and Quantum Chemical Studies

Publication details

Journal / source
Optics Letters
Volume
51
Issue
7
Pages
1752–1752
Publication date
5 March 2026
Language
EN