Mid-infrared nonlinear optical materials for ultrafast sources: opinion

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Authors: Peter G. Schunemann, Kevin T. Zawilski, Jani Jesenovec, Eric D. Readinger
Cited by: 4
References: 33

Abstract

High-performance nonlinear optical (NLO) materials are essential for shifting ultrafast laser sources deep into the mid-infrared, especially for spectroscopic applications aimed at identifying species in the molecular fingerprint region (6.7–20 μm). Traditional oxide NLO crystals are limited to output wavelengths below 5 μm, but non-oxide semiconductors like ZGP, CSP, OP-GaAs, and OP-GaP offer deep infrared transparency, high nonlinearities, and broadband tunability. We review essential property requirements, compare materials of choice in two distinct classes - bulk birefringent crystals and quasi-phase-matched semiconductors - cite key ultrafast laser demonstrations, and identify emerging new materials and future directions in the field.

Fields of Study & Subjects

Nonlinear Photonic Systems Photorefractive and Nonlinear Optics Advanced Fiber Laser Technologies

Publication details

Journal / source
Optical Materials Express
Publisher
Optica Publishing Group
Volume
16
Issue
3
Pages
656–656
Publication date
19 February 2026
Language
EN