Discovery of high-temperature charge order and time-reversal symmetry-breaking in the kagome superconductor YRu$_3$Si$_2$

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Authors: P. Král, J. N. Graham, V. Sazgari, Igor Plokhikh, A. Lukovkina, O. Gerguri, I. Biało, Andrin Doll, Leonardo Martinelli, Jens Oppliger, S. S. Islam, M. Spitaler
+13 more K. Wang, M. Salamin, H. Luetkens, Rustem Khasanov, M. v. Zimmermann, J. -X. Yin, Ziqiang Wang, J. Chang, B. Monserrat, Dariusz Jakub Gawryluk, Fabian O. von Rohr, Sun-Woo Kim, Zurab Guguchia
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Abstract

Identifying high-temperature unconventional charge order and superconductivity in kagome systems is crucial for understanding frustrated, correlated electrons and enabling future quantum technologies. Here, we report that the kagome superconductor YRu$_3$Si$_2$ hosts an exceptional interplay of charge order, magnetism, and superconductivity, revealed through a comprehensive suite of muon spin rotation (μSR), magnetotransport, X-ray diffraction, and density functional theory (DFT). We identify a high-temperature charge-ordered state with propagation vector (1/2,0,0) and a record onset temperature of 800 K, unprecedented in kagome systems and quantum materials more broadly. μSR measurements further reveal time-reversal symmetry-breaking below 25 K and field-induced magnetism near 90 K, features mirrored in the magnetoresistance, which reaches 45% at low temperatures. Band-structure calculations show two van Hove singularities near the Fermi level, including one within a flat band. At low temperatures, YRu$_3$Si$_2$ becomes superconducting below Tc = 3.4 K with either two full isotropic gaps or an anisotropic nodeless gap. These results establish YRu$_3$Si$_2$ as a prime platform for studying correlated kagome physics.

Fields of Study & Subjects

Advanced Condensed Matter Physics Physics of Superconductivity and Magnetism Rare-earth and actinide compounds

Publication details

Journal / source
DESY Publication Database (PUBDB) (Deutsches Elektronen-Synchrotron)
Publication date
1 January 2026
Language
EN