Magnetic states of the Kondo lattice Ce$_2$PdSi$_3$ and their pressure evolution

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Authors: Yanan Zhang, Zhaoyang Shan, Jiawen Zhang, Kaixin Ye, Yongjian Li, Dajun Su, Pascal Manuel, Dmitry D. Khalyavin, Devashibhai Thakarshibhai Adroja, Daniel Alexander Mayoh, Geetha Balakrishnan, Yu Liu
+2 more M. Smidman, Huiqiu Yuan
Cited by: 0

Abstract

Frustrated Kondo lattices are ideal platforms for exploring unconventional forms of quantum criticality, as well as magnetism and other emergent phases. Here we report the magnetic properties of the candidate frustrated heavy fermion compound Ce$_2$PdSi$_3$, and map their evolution upon applying magnetic fields and hydrostatic pressure. We find that at ambient pressure Ce$_2$PdSi$_3$ exhibits two distinct magnetic phase transitions, a ferromagnetic-like transition at $T_{\mathrm{M1}}=3.8$ K and an incommensurate antiferromagnetic transition at $T_{\mathrm{M2}}=2.9$ K. Upon applying pressure, $T_{\mathrm{M1}}$ is continuously suppressed and becomes undetectable above 4.2 GPa, whereas $T_{\mathrm{M2}}$ increases and remains robust up to at least 7.5 GPa. The observed pressure evolution of magnetic order in Ce$_2$PdSi$_3$ suggests the presence of competing magnetic orders, and cannot be simply encapsulated by the Doniach phase diagram, motivating further investigations for its origin, including discerning the role of geometric frustration.

Fields of Study & Subjects

Rare-earth and actinide compounds Advanced Condensed Matter Physics Magnetic and transport properties of perovskites and related materials

Publication details

Journal / source
arXiv (Cornell University)
Publication date
28 January 2026
Document type
Preprint