Ultrafast Decoherence of Charge Density Waves in K$_{0.3}$MoO$_{3}$

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Authors: Winkler, Rafael T., Larissa Boie, Yunpei Deng, Matteo Savoini, Serhane Zerdane, Abhishek Nag, Sabina Gurung, Davide Soranzio, Tim Suter, Vladimir Ovuka, Janine Zemp, Elsa Abreu
+11 more Simone Biasco, Roman Mankowsky, E. J. Divall, Alexander R. Oggenfuss, Mathias Sander, Christopher Arrell, Danylо Babich, Henrik Till Lemke, U. Staub, Jure Demsar, Steven L. Johnson
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Abstract

Recent works have suggested that transient suppression of a charge density wave (CDW) by an ultra-short excitation can lead to an inversion of the CDW phase. We experimentally investigate the dynamics of the CDW in K$_{0.3}$MoO$_{3}$ by time resolved x-ray diffraction after excitation with optical pulses. Our results indicate a transient inversion of the CDW phase close to the surface that evolves into a highly disordered state in less than one picosecond. Numerical simulations solving the Ginzburg-Landau equation including disorder from strong pinning defects reproduce our main observations. Our findings highlight the critical role of disorder in schemes for coherent control in condensed matter systems.

Fields of Study & Subjects

Organic and Molecular Conductors Research Advanced Condensed Matter Physics Physics of Superconductivity and Magnetism

Publication details

Journal / source
arXiv (Cornell University)
Publication date
28 January 2026
Document type
Preprint