Probing Interfacial Spin Dynamics and Temperature Dependent Asymmetry in Spin Pumping Across Ni80Fe20/Cu/Cr1.12Te2 Interfaces

Spin transfers in magnetic multilayers offers a promising pathway toward ultrafast, energy-efficient spintronic devices. In this study, we investigate the interfacial spin pumping and temperature-dependent spin current exchange in a Cr1.12Te2/Cu/Ni80Fe20 (Py)(FM1/NM/FM2) trilayer structure. Using broadband and cryogenic ferromagnetic resonance (FMR) measurements, we investigate key magnetization dynamical parameters, including the effective Gilbert damping factor, effective magnetic fields, interfacial spin mixing conductance, and spin current density. Efficient spin angular momentum transfers from Py to Cr1.12Te2 are observed at room temperature. At lower temperatures, the enhanced linewidth reflects temperature dependent spin pumping effects occurring at distinct precession frequencies of the ferromagnetic layers. Notably, the absence of interfacial Damping indicates that spin pumping can be modulated by controlling the net spin current flow. These findings offer critical insight into temperature-dependent tunable spin transport mechanisms in magnetic multilayers, highlighting their potential for next-generation spintronic applications.