Kondo Reshapes Multiple Orders in a $5f$ van der Waals Material

Read full text
Authors: Gal Tuvia, Ruizhe Kang, Diana Golovanova, Yuqian Chen, Yidi Wang, Zeyu Ma, Mengke Liu, Carly Grossman, Suk Hyun Sung, Justin Shotton, Jiahui Zhu, David Alonso Martinez
+5 more Ismail El Baggari, Binghai Yan, Dirk K. Morr, Sheng Ran, Jennifer E. Hoffman
Cited by: 0

Abstract

Electron interactions can drive magnetism, superconductivity, and topology. However, the realization of these phases remains limited in van der Waals materials, and the full landscape of strong correlations remains uncharted in any context. While interactions between conduction electrons and localized spins yield a well-known competition between heavy fermions (Kondo hybridization) and magnetic order (RKKY exchange), such spin-driven competition represents only part of the correlated electron phase diagram. Here we demonstrate that a heavy-fermion state can also compete with charge order, such as the charge density wave (CDW) state typical in the van der Waals $4f$ rare-earth tritellurides (RTe$_3$). We exploit the spatially-extended $5f$ orbitals of $β$-UTe$_3$ to enhance Kondo hybridization compared to its isostructural RTe$_3$ cousins. Our scanning tunneling spectroscopy on $β$-UTe$_3$ shows Fano resonances characteristic of the heavy fermion state, while our quasiparticle interference imaging reveals the disappearance of Fermi-level nesting and the appearance of flat bands. We extend the tritelluride tight-binding model to include Kondo coupling and quantify the Fermi surface reconstruction. Consistent with the destruction of nesting, we observe no CDW in $β$-UTe$_3$. Our expansion of the Kondo phase diagram beyond spin-mediated competition opens new possibilities for proximity-induced phase engineering in correlated van der Waals heterostructures.

Fields of Study & Subjects

Rare-earth and actinide compounds Physics of Superconductivity and Magnetism Advanced Condensed Matter Physics

Publication details

Journal / source
arXiv (Cornell University)
Publication date
25 February 2026
Language
EN
Document type
Preprint