Persistent short-range charge correlations revealed by ultrafast melting of electronic order in YBa$_2$Cu$_3$O$_{6+x}$

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Authors: C. Seo, L. Shen, Alexander N. Petsch, Scott Wandel, Vincent Esposito, J. D. Koralek, Georgi L. Dakovski, M-F. Lin, S. P. Moeller, W. F. Schlotter, Alexander H. Reid, Michael P. Minitti
+9 more Ruixing Liang, D. A. Bonn, W. N. Hardy, A. Damascelli, C. Giannetti, E. H. da Silva Neto, Joshua J. Turner, Fabio Boschini, Giacomo Coslovich
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References: 1

Abstract

Charge density waves (CDW) are ubiquitous in the complex phase diagram of cuprate superconductors and exhibit both short- and long-range correlations. Using time-resolved resonant X-ray scattering, we investigate the photo-induced dynamics of CDW in YBa$_2$Cu$_3$O$_{6.67}$. We discover an excitation threshold ($Φ$$_\mathrm{C}$ $\approx$ 65 $μ$J/cm$^2$) above which long-range CDW disappear, revealing a persistent CDW peak with short-range correlation length. Ultrafast photo-excitation promptly uncovers this residual short-range CDW correlations, appearing within $\approx$ 0.2 ps. Long-range CDW coherence recovers within $\approx$ 0.6 ps, while the peak intensity remains partially suppressed. We rationalize the dichotomic behavior in the fluence and temporal dependencies as the signature of two coexisting CDW peaks, arising from short- and long-range correlations, which we disentangle through their distinct response to photo-excitation. We provide evidence that the collapse of long-range correlations is driven by an electronic process, while short-range correlations are characterized by distinct timescales and stiffness against photo-excitation. This approach establishes ultrafast X-ray scattering as an effective tool for disentangling coexisting density waves and correlations in quantum materials.

Fields of Study & Subjects

Physics of Superconductivity and Magnetism Advanced Condensed Matter Physics Electronic and Structural Properties of Oxides

Publication details

Journal / source
arXiv (Cornell University)
Publication date
11 March 2026
Language
EN
Document type
Preprint