Data for "Interradical motion can push magnetosensing precision towards quantum limits"
Abstract
Abstract: Magnetosensitive spin-correlated radical-pairs (SCRPs) offer a promising platform for noise-robust quantum metrology. However, unavoidable interradical interactions, such as electron-electron dipolar and exchange couplings, alongside deleterious perturbations resulting from intrinsic radical motion, typically degrade their potential as magnetometers. In contrast to this, we show how structured molecular motion modulating interradical interactions in a live chemical sensor in cryptochrome can, in fact, increase sensitivity and, more so, push precision in estimating magnetic field directions closer to the quantum Cramér–Rao bound, suggesting near-optimal metrological performance. Remarkably, this approach to optimality is amplified under environmental noise and persists with increasing complexity of the spin system, suggesting that perturbations inherent to such natural systems have enabled them to operate closer to the quantum limit to more effectively extract information from the weak geomagnetic field. This insight opens the possibility of channeling the underlying physical principles of motion-induced modulation of electron spin-spin interactions towards devising efficient handles over emerging molecular quantum information technologies. This repository collects the data plotted in the associated manuscript "Interradical motion can push magnetosensing precision towards quantum limits", by Luke D. Smith, Farhan T. Chowdhury, Jonas Glatthard, and Daniel R. Kattnig.
Fields of Study & Subjects
Electron Spin Resonance Studies
Quantum Information and Cryptography
Magnetism in coordination complexes
Publication details
- Journal / source
- Figshare
- Publication date
- 1 January 2026
- Document type
- Dataset