Excited-state vibronic coherences with mixing of core-ligand character promote hot-carrier cooling in oleate-capped CdSe quantum dots

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Authors: Warren Beck, Mengliang Zhang, Kevin Cavey, Benjamin G. Levine, P. Gregory Van Patten, Nila Mohan T. M., Caitlin V. Hetherington, Shanu A. Shameem, Chase H. Leslie
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Abstract

We present herein a multidimensional electronic spectroscopy study (2DES and 3DES) of vibronic coherences in CdSe quantum dots (QDs) showing that mid-frequency vibrations of the surface-capping oleate ligands promote hot-carrier cooling on the

Fields of Study & Subjects

Quantum Dots Synthesis And Properties Spectroscopy and Quantum Chemical Studies Semiconductor Quantum Structures and Devices

Publication details

Journal / source
AIP Publishing
Publication date
1 January 2026
Language
EN